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• W2045689310 abstract "Considering as an example the 2A+B2→2AB reaction occurring on the surface of a catalyst, we demonstrate that heterogeneous reactions may exhibit oscillatory behavior at isothermal conditions if the bistability of the nonoscillatory surface kinetics is combined with diffusion limitations in the gas phase. Exploring this general phenomenon for a spherical catalyst, we derive necessary conditions for its observation, estimate analytically the period of oscillations, and study numerically in detail both transient and sustained oscillatory regimes. In addition, we show that one can obtain damped oscillations in the regions where the necessary conditions for sustained oscillatory kinetics are not fulfilled (in this case the period of the oscillations monotonically increases with increasing time, and then the oscillations disappear). The requirements on experimental systems to observe this phenomenon are also discussed." @default.
• W2045689310 created "2016-06-24" @default.
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• W2045689310 date "1997-02-22" @default.
• W2045689310 modified "2023-09-27" @default.
• W2045689310 title "Oscillatory surface reaction kinetics due to coupling of bistability and diffusion limitations" @default.
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• W2045689310 doi "https://doi.org/10.1063/1.473054" @default.
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