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• W2045721844 startingPage "2278" @default.
• W2045721844 abstract "Photon emission from a metal surface (Au and Pt) induced by electron-transfer reactions was observed in an electrolyte solution containing solvated electrons. The quantum efficiency ensuremath{Phi} increases as the electrode potential ${mathit{U}}_{mathit{w}}$ becomes positive. The high-energy threshold of the spectrum, ${mathit{E}}_{mathrm{th}}$, increases linearly with increasing ${mathit{U}}_{mathit{w}}$ at the rate of 1 eV/V. The relaxation energy of solvated electrons in the electrolyte solution is estimated from the values of ${mathit{E}}_{mathrm{th}}$ and ${mathit{U}}_{mathit{w}}$. The peak energy ${mathit{E}}_{mathit{p}}$ of the spectrum also increases as ${mathit{U}}_{mathit{w}}$ becomes positive although the magnitude of the shift is much smaller than that of ${mathit{E}}_{mathrm{th}}$. ${mathit{E}}_{mathit{p}}$ and the low-energy threshold ${mathit{E}}_{mathit{l}}$ of the spectrum are metal dependent. The emitted-photon spectra are simulated by considering the transition between bulk band states of the metal while ignoring k-vector conservation. The simulated results are compared with experiment and the validity of this model is discussed." @default.
• W2045721844 created "2016-06-24" @default.
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• W2045721844 date "1993-01-15" @default.
• W2045721844 modified "2023-09-23" @default.
• W2045721844 title "Observation and mechanism of photon emission at metal-solution interfaces" @default.
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• W2045721844 doi "https://doi.org/10.1103/physrevb.47.2278" @default.
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