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• W2045853872 abstract "Dynamic voltammetric experiments on a number of European river water samples reveal the presence of labile zinc(II) complexes with stability constants in the range between 106.4 and 107 M-1. Theoretical reconstruction of the labilities on the basis of the elementary association/dissociation rate constants confirms the experimental findings. Taking into account (i) the differences in diffusion coefficients between free metal ions and metal complexes, and (ii) the lability of the complexes, the distribution of zinc(II) over free metal and complexed species is found to be roughly 30% and 70%, respectively. Consequently the operational bioavailability of zinc(II), i.e., the flux of zinc(II) into an organism, is reduced to 30% if the actual interfacial uptake process is rate-determining. The reduction amounts to 50% if the diffusional supply of zinc(II) to the biointerphase is rate-determining." @default.
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• W2045853872 date "1998-11-04" @default.
• W2045853872 modified "2023-10-18" @default.
• W2045853872 title "Speciation and Lability of Zinc(II) in River Waters" @default.
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• W2045853872 doi "https://doi.org/10.1021/es9801590" @default.
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