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- W2046396963 abstract "A fluorophore is converted from its ground state A to an electronically excited state A* by absorption of a photon hνex. A* decays to A by fluorescence, with a lifetime τ. It is quenched by collision with quencher Q at a diffusion controlled rate k[Q]. We suppose that A and Q are capable of reacting to form a complex AQ, even in the absence of the excitation. AQ forms at a diffusion controlled rate kf[Q] and decays at a rate kb. It is assumed that the quencher concentration is large enough so their depletion in the forward reaction of the final step can be neglected. The Stern–Volmer law is derived for the above four step chemical mechanism; the theory being given to all orders in the concentration of the quenchers. The results are compared with the concentration dependence proposed by Felderhof and Deutch. It is concluded that the predictions of the present work should be amenable to experimental test." @default.
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- W2046396963 date "1983-06-01" @default.
- W2046396963 modified "2023-10-16" @default.
- W2046396963 title "Finite concentration fluorescence quenching in the presence of diffusion" @default.
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- W2046396963 doi "https://doi.org/10.1063/1.444656" @default.
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