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• W2046759527 abstract "Abstract The interaction between molecular oxygen and the metal atom in two Co(II) complexes with bis(diacetylmonoxime-imino)propane-1,3 ( A ) and with the related ligand obtained from cobaloxime by substitution of both the O-H ⋯ O bridges with the -BF 2 -group ( B ) is investigated using electrochemical and spectroelectrochemical techniques. Notwithstanding the stability of the Co(II) complex B in air, the results suggest the formation of a dioxygen adduct as an unstable intermediate in the electrocatalytic reduction of molecular oxygen in the presence of either A or B . Furthermore, the oxygenation ratio at a given p O 2 appears to be quite different for the homogeneous reaction of A in the Co(II) oxidation state in bulk as compared with either the electrogenerated Co(II) (from complex A ) on the electrode surface or the Co(II) complex B ." @default.
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• W2046759527 date "1991-11-01" @default.
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• W2046759527 title "Electrochemical investigation of dioxygen interaction with two cobalt chelates in solution and at the electrode surface" @default.
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• W2046759527 doi "https://doi.org/10.1016/0022-0728(91)85303-7" @default.
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