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- W2046765361 abstract "The intramolecular Diels−Alder (IMDA) reactions of C(8)-substituted decatrienoates have been studied. The stereospecific formation of 11 via an endo-boat-9 transition state attests to the powerful directing influence of a C(8) substituent in the IMDA of decatrienoate. In addition, the contrasting observations that stereospecific 9 → 11 occurs at room temperature while the nor-tert-butyl substrate (4a) requires 125 °C/5 h reaction conditions and produces a 60:40 mixture of diastereomers provide clear evidence that a bulky C(8) substituent is a powerful conformational activator of the IMDA." @default.
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- W2046765361 date "2000-06-01" @default.
- W2046765361 modified "2023-10-16" @default.
- W2046765361 title "Intramolecular Diels−Alder Reactions of Decatrienoates: Remote Stereocontrol and Conformational Activation<sup>1</sup>" @default.
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- W2046765361 doi "https://doi.org/10.1021/ol005886q" @default.
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