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• W2046918100 abstract "Equilibrium and rate constants of the self-association of methylene blue and pyronine G in aqueous solutions (water and water/methanol mixtures) are reported for pressures up to 200 MPa at T = 20°C and 30°C. The kinetic measurements were performed in a high pressure cable temperature-jump apparatus. The volumes of reaction determined from the pressure dependence of the association constants are negative (–9.0 to –13.5 cm3 mol−1) for all reactions. From the pressure dependence of the rate constants the volumes of activation are found to be slightly negative for the forward reaction (±0 to –5.3 cm3 mol−1) and positive for the reverse direction (+ 4.3 to + 13.3 cm3 mol−1). The volumes of reaction of the two intermediate steps of the self-association (i.e. formation of the encounter complex and rearrangement of the complex to form the dimer) are calculated by using the theory of diffusion controlled reactions. The resulting volume profiles of the reactions are discussed in view of the specific role of water as solvent." @default.
• W2046918100 created "2016-06-24" @default.
• W2046918100 creator A5080146949 @default.
• W2046918100 date "1984-02-01" @default.
• W2046918100 modified "2023-09-25" @default.
• W2046918100 title "The Effect of Pressure on the Self-Association of Dyes in Aqueous Solutions Studied by Cable Temperature-Jump Relaxation Spectroscopy" @default.
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• W2046918100 doi "https://doi.org/10.1002/bbpc.19840880207" @default.
• W2046918100 hasPublicationYear "1984" @default.
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