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- W2047129478 abstract "The kinetics of the thermal undoping process of doped poly(3-butylthiophenes) and poly(3-octylthiophenes) have been studied using optical spectroscopy. The process is faster with higher temperatures and with longer side chains. No simple reaction kinetic model has been found. The process can be described using a master-plot technique. This master plot can be fitted with a Williams-Landell-Ferry (WLF)-type equation. The coupling of free volume mechanisms, as evidenced in the fit with the WLF equation, and thermal undoping supports our interpretation of the thermal undoping as due to thermally induced disorder in the side chains, main chain torsion and, consequently, reduction of the polymer due to the increased oxidation potential in the twisted state. To enhance stability in the doped polymer, suppression of side chain mobility or precautions towards their influence on dopant geometry and main chain geometry is suggested." @default.
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- W2047129478 title "A kinetic study of thermal undoping in the poly(3-alkylthiophenes)" @default.
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- W2047129478 doi "https://doi.org/10.1016/0379-6779(92)90046-l" @default.
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