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- W2047349623 abstract "Zeolite-templated carbon (ZTC) materials were synthesized, characterized, and evaluated as potential hydrogen storage materials between 77 and 298 K up to 30 MPa. Successful synthesis of high template fidelity ZTCs was confirmed by X-ray diffraction and nitrogen adsorption at 77 K; BET surface areas up to ∼3600 m2 g–1 were achieved. Equilibrium hydrogen adsorption capacity in ZTCs is higher than all other materials studied, including superactivated carbon MSC-30. The ZTCs showed a maximum in Gibbs surface excess uptake of 28.6 mmol g–1 (5.5 wt %) at 77 K, with hydrogen uptake capacity at 300 K linearly proportional to BET surface area: 2.3 mmol g–1 (0.46 wt %) uptake per 1000 m2 g–1 at 30 MPa. This is the same trend as for other carbonaceous materials, implying that the nature of high-pressure adsorption in ZTCs is not unique despite their narrow microporosity and significantly lower skeletal densities. Isoexcess enthalpies of adsorption are calculated between 77 and 298 K and found to be 6.5–6.6 kJ mol–1 in the Henry’s law limit." @default.
- W2047349623 created "2016-06-24" @default.
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- W2047349623 date "2012-06-19" @default.
- W2047349623 modified "2023-10-11" @default.
- W2047349623 title "Zeolite-Templated Carbon Materials for High-Pressure Hydrogen Storage" @default.
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- W2047349623 doi "https://doi.org/10.1021/la302050m" @default.
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