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• W2047362955 endingPage "7792" @default.
• W2047362955 startingPage "7785" @default.
• W2047362955 abstract "Ultrafine monodisperse gold nanoparticles (AuNPs) were synthesized by an elegant sputtering of gold onto 1- n-butyl-3-methylimidazolium hexafluorophosphate (BMI-PF(6)) ionic liquid. It was found that the BMI-PF(6) supramolecular aggregates were loosely coordinated to the gold nanoparticles and were replaceable with thiol molecules. The self-assembly of BMI-PF(6)-stabilized AuNPs onto a (3-mercaptopropyl)trimethoxysilane (MPS)-functionalized silicon surface in 2D arrays, followed by dodecanethiol (DDT) treatment, have been demonstrated using X-ray photoelectron spectroscopy, field emission scanning electron microscopy, and contact angle measurements. DDT treatment of tethered AuNPs revealed two types of interactions between AuNPs and the MPS-functionalized surface: (a) AuNPs anchor through Au-S chemisorption linkage resulting in strong immobilization and (b) some of the AuNPs are supported by physisorption, driven by BMI-PF(6). The attachment of these particles remains unchanged with sonication. The replacement of BMI-PF(6) aggregates from physisorbed AuNPs with DDT molecules advances the dilution of their interaction with the MPS-functionalized surface, and they subsequently detach from the silicon surface. The present finding is promising for the immobilization of ionic liquid-stabilized nanoparticles, which is very desirable for electronic and catalytic device fabrication. Additionally, these environmentally friendly AuNPs are expected to replace conventional citrate-stabilized AuNPs." @default.
• W2047362955 created "2016-06-24" @default.
• W2047362955 creator A5006247568 @default.
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• W2047362955 date "2008-06-24" @default.
• W2047362955 modified "2023-09-25" @default.
• W2047362955 title "Self-Assembly of Ionic Liquid (BMI-PF₆)-Stabilized Gold Nanoparticles on a Silicon Surface: Chemical and Structural Aspects" @default.
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• W2047362955 doi "https://doi.org/10.1021/la800678m" @default.
• W2047362955 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18572958" @default.
• W2047362955 hasPublicationYear "2008" @default.
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