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- W2047540904 abstract "A simple calculation method is presented which allows for estimation of the fractions of different iron species in Fe-ZSM-5 based on statistical considerations. Under the assumption of uniformly distributed iron, the probability with which Fe–O–Fe bridged and higher nuclear Fe-species are formed in a Fe-ZSM-5 sample may be calculated based on a simple Poisson distribution. The results of these calculations were compared with DR-UV/vis and DRIFT spectroscopy measurements on a variety of Fe-ZSM-5 samples with different Fe/Al ratios. Moreover, the calculated concentration profiles were checked with literature data from other studies. It is shown that the fractions of different iron species in Fe-ZSM-5 can be estimated by this calculation method with satisfactory accuracy, provided that the metal-exchange process resulted in a uniform distribution of iron in the zeolite. The method may be useful for verifying of analytical results, understanding of observed activity patterns and may facilitate the identification of activity–structure relationships." @default.
- W2047540904 created "2016-06-24" @default.
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- W2047540904 date "2010-01-31" @default.
- W2047540904 modified "2023-09-26" @default.
- W2047540904 title "Estimation of the fractions of different nuclear iron species in uniformly metal-exchanged Fe-ZSM-5 samples based on a Poisson distribution" @default.
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- W2047540904 doi "https://doi.org/10.1016/j.apcata.2009.11.012" @default.
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