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- W2047643863 abstract "The electronic dephasing of large molecules in solution is investigated with three-pulse photon echoes generated by 6-fs optical pulses. The observed dephasing behavior, which is analyzed with a model based on a stochastic coupling of the molecules with their heat bath, is clearly shown to be non-Markovian. Moreover, the correlation function of the fluctuations asymptotically approaches an exponential with characteristic times varying from 20 to 80 fs, depending on the solvent environment." @default.
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- W2047643863 date "1991-03-04" @default.
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- W2047643863 title "Non-Markovian dephasing of molecules in solution measured with three-pulse femtosecond photon echoes" @default.
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- W2047643863 doi "https://doi.org/10.1103/physrevlett.66.1138" @default.
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