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• W2047712501 abstract "The high plutonium, hypo-stoichiometric fuel exists as two phase system at low temperatures. The partial phase diagram of (U,Pu)O2−x with two coexisting cubic phases was extensively investigated in this work using theoretical models. The critical temperature of the miscibility gap varies with Pu/M and O/M of the system. Based on the similar miscibility gap behaviour observed in PuO2−x system and the experimental data available on the phase boundaries of (U,Pu)O2−x for various Pu/M, some semi-empirical relationships and solution models were developed. With the help of these relationships, ternary isothermal sections of the miscibility gap, O/M at different temperatures and the critical temperature of the miscibility gap of (U,Pu)2−x for different Pu/M values were calculated. These calculated values were compared with the available literature data." @default.
• W2047712501 created "2016-06-24" @default.
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• W2047712501 date "2009-03-01" @default.
• W2047712501 modified "2023-09-23" @default.
• W2047712501 title "Phase diagram analysis of (U,Pu)O2−x sub-system" @default.
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• W2047712501 doi "https://doi.org/10.1016/j.jnucmat.2008.10.017" @default.
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