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• W2047776799 abstract "The third CH stretching vibration overtone (4νCH) of the acetylene molecule has been a prototype for intra-molecular dynamics studies. Using a sensitive cavity ring-down spectrometer calibrated with precise atomic transitions, the absolute line frequencies of 50 lines of this band have been determined with sub-MHz accuracy, or relatively 2 × 10−9. The accuracy is also confirmed by the combination differences between the transitions sharing the same upper level. The improved accuracy, two orders of magnitude better than previous studies, allows us to reveal finer ro-vibrational couplings. Fitting of the rotational energies indicates that the J-dependent interactions take place after J &gt; 7. The precise line positions present useful confinements to the models of the intra-molecular interactions of the acetylene molecule." @default.
• W2047776799 created "2016-06-24" @default.
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• W2047776799 date "2013-01-07" @default.
• W2047776799 modified "2023-10-17" @default.
• W2047776799 title "The 4ν<i>CH</i> overtone of 12C2H2: Sub-MHz precision spectrum reveals perturbations" @default.
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• W2047776799 doi "https://doi.org/10.1063/1.4773473" @default.
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• W2047776799 hasPublicationYear "2013" @default.
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