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• W2047999280 abstract "Transions among melt, glass, and crystal states are modeled phenomenologically by integrating notions from chemical kinetics with a Landau-type generalization of the concept of affinity. The model naturally captures the melt → glass, melt → crystal, and glass → crystal transitions. The Landau terms in a free energy ansatz allow for the prediction of domains of various types of molecular orderings. A simple “symmetric conflict” model is considered as a concrete realization of the approach. This model explicitly demonstrates the existence of a higher lying glasslike free energy well that is kinetically favored over a deeper-lying crystal well. Quenching to the glass state and annealing to the crystal state are shown to follow naturally. The spontaneous creation of ordering domains is proposed to be a self-organizing process. The formalism may be generalized to allow for the analysis of chemically complex, multicomponent systems." @default.
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• W2047999280 date "1997-10-01" @default.
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• W2047999280 title "Glass Transitions: A Chemical Kinetic/Landau Theory" @default.
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• W2047999280 doi "https://doi.org/10.1021/jp962453p" @default.
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