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- W2048005029 abstract "Abstract The stereoselectivities obtained in Lewis acid‐promoted Mukaiyama aldol additions and Sakurai allylations of mono‐, and syn ‐ and anti ‐disubstituted aldehydes possessing various polar α‐ and β‐substituents under non‐chelating conditions are presented. The stereochemical outcome in the nucleophilic addition to α‐substituted aldehydes containing an α‐benzyloxy, α‐fluoro or α‐sulfonamide substituent are accurately predicted by current stereoinduction models. In contrast, the selectivitites obtained from addition of sterically demanding nucleophiles to α‐chloro‐substituted aldehydes cannot be rationalized by the same models and an alternative is discussed. The stereochemichal outcome in the additions to α,β‐disubstituted aldehydes is more complex and cannot be predicted using current models." @default.
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- W2048005029 date "2011-08-01" @default.
- W2048005029 modified "2023-10-06" @default.
- W2048005029 title "Diastereoselective Nucleophilic Addition to Aldehydes with Polar α- and α,β-Substituents" @default.
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- W2048005029 doi "https://doi.org/10.1002/adsc.201100173" @default.
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