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• W2048570071 abstract "Methyl chloride (CH 3 Cl) is the most abundant, natural, chlorine‐containing gas in the atmosphere, with oceans and biomass burning as major identified sources. Estimates of global emissions suffer from large uncertainties, mostly for the tropics, partly due to a lack of measurements. We present analyses of whole‐air canister samples for selected nonmethane hydrocarbons and chlorocarbons. The samples were collected from an aircraft during the Indian Ocean Experiment (INDOEX) campaign over the northern Indian Ocean in February and March 1999. The CH 3 Cl results are correlated to selected nonmethane hydrocarbons and in situ measurements of carbon monoxide (CO) and acetonitrile (CH 3 CN). We relate high mixing ratios of ∼750 pmol mol −1 of CH 3 Cl to biomass burning, as observed in polluted air masses from India and Southeast Asia. We infer a relatively high enhancement ratio relative to CO, ΔCH 3 Cl/ΔCO ≈1.74 ± 0.21 × 10 −3 mol mol −1 . The CH 3 Cl levels relate to the extensive biofuel use in India and Southeast Asia, notably the burning of agricultural waste and dung with a comparatively high chlorine content. It appears that CH 3 Cl emissions from biofuel consumption in India and Southeast Asia have been underestimated in the past. Furthermore, we observed enhanced dichloromethane (CH 2 Cl 2 ) and trichloromethane (CHCl 3 ) levels, correlating with high CO, acetylene (C 2 H 2 ) and CH 3 Cl, indicating that biomass burning is a small but significant source of these species." @default.
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• W2048570071 date "2002-09-04" @default.
• W2048570071 modified "2023-10-17" @default.
• W2048570071 title "Methyl chloride and other chlorocarbons in polluted air during INDOEX" @default.
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• W2048570071 doi "https://doi.org/10.1029/2001jd001121" @default.
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