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• W2048650511 abstract "The coordination of [(η-Cp)2Pb] and [(η-Cp)2Sn] by bidentate Lewis-base ligands gives the first examples of adducts of neutral p-block metallocenes. Ab initio MO calculations of [(η-Cp)2Pb·TMEDA] (1) (TMEDA = (Me2NCH2)2), [Cp2Pb·4,4‘-Me2bipy] (2) (4,4‘-Me2bipy = 4,4‘-dimethylbipyridine), and the new complex [(η-Cp)2Sn·TMEDA] (3) confirm that despite the presence of longer Pb−N and Sn−N bonds in the solid-state structures of the TMEDA adducts, the association of TMEDA with the metallocenes is more favorable than with 4,4‘-Me2bipy. This finding is a consequence of the greater reorganization energy of 4,4‘-Me2bipy compared to TMEDA. The low association energies of these species can be rationalized in terms of metal lone pair/ligand lone pair repulsion." @default.
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• W2048650511 date "1998-06-25" @default.
• W2048650511 modified "2023-10-12" @default.
• W2048650511 title "Weakly Bonded Lewis Base Adducts of Plumbocene and Stannocene: A Synthetic and Calculational Study" @default.
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• W2048650511 doi "https://doi.org/10.1021/om980077k" @default.
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