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- W2048651107 startingPage "354" @default.
- W2048651107 abstract "The large chemical shifts recently observed in Mossbauer absorption experiments on ${mathrm{Au}}^{197}$ are explained on the basis of Coulombic interaction between the $6s$ electron of gold and the $3{s}_{frac{1}{2}}$ and $2{d}_{frac{3}{2}}$ protons. A first-order perturbation calculation is made, using the Coulombic potential within the nucleus due to the $6s$ electron. Proton wave functions derived from harmonic-oscillator, square-well, and Woods-Saxon nuclear potentials are treated. The latter two potentials yield results that are in reasonable accord with experiment. This model can afford a sensitive comparison of nuclear potentials as well as a determination of the $s$ conduction-electron density on impurity atoms. In particular, this calculation discriminates against the harmonic-oscillator potential and shows that the $6s$ electron density on a gold impurity atom in several hosts is higher than in pure gold. These results also indicate that the $3{s}_{frac{1}{2}}$ proton subshell is filled in the ground state of ${mathrm{Au}}^{197}$." @default.
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- W2048651107 date "1961-10-15" @default.
- W2048651107 modified "2023-09-24" @default.
- W2048651107 title "Interpretation of the Isomeric Chemical Shifts in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:mrow><mml:mi mathvariant=normal>Au</mml:mi></mml:mrow><mml:mrow><mml:mn>197</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math>" @default.
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- W2048651107 doi "https://doi.org/10.1103/physrev.124.354" @default.
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