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• W2048651429 abstract "Two-photon-photoemission (2PPE) spectroscopy is employed to characterize electronic states of a bilayer C6H6/Cu{111} system at 85 K. The unoccupied benzene π* e2u state is observed with a binding energy of 4.6 eV above the Fermi level. This result agrees with inverse-photoemission (IPE) data and provides a case where the determination of the binding energy is identical for 2PPE and IPE. The π* e2u state is assigned in the 2PPE scheme as a final state which is the first observed final state in 2PPE of adsorbate-surface systems. The dependence of the electron dynamics on the morphology of an incomplete adsorption layer is also investigated. Two (n=1)-like image potential states A and B are observed which presumably originate from two different C6H6 adsorption geometries in the bilayer regime. The two image states A and B are characterized by electron effective masses of 1.1 and 1.9 me, binding energies of 3.30 and 3.45 eV above the Fermi level, and lifetimes of 40 and 20 fs, respectively. The dielectric con..." @default.
• W2048651429 created "2016-06-24" @default.
• W2048651429 creator A5010170160 @default.
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• W2048651429 date "1998-11-22" @default.
• W2048651429 modified "2023-09-24" @default.
• W2048651429 title "Electronic states of the C6H6/Cu{111} system: Energetics, femtosecond dynamics, and adsorption morphology" @default.
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• W2048651429 doi "https://doi.org/10.1063/1.477468" @default.
• W2048651429 hasPublicationYear "1998" @default.
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