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- W2048654990 abstract "The excitation spectrum of the XeCl (B, v' = 0–21) molecule was determined in a wide range of wave-lengths (315–275 nm). The molecules were formed as a result of flash photolysis by excimer laser radiation of gaseous Xe—Cl2 mixtures of natural isotopic composition. They were then pumped by light from a frequency-tunable dye laser. A comparison of the intensities of free—bound and bound—bound transitions was used to estimate the rate constant of photoassociation, regarded as recombination of Xe and Cl atoms in which a photon acts as the third body: the rate was found to be ≈ 6×10-29 cm6 s-1 at λ ≈ 310.5 nm. A comparative analysis of the dependence of the intensity of the luminescence emitted by XeCl (C—A) and Xe2Cl*, pumped in the region of the long-wavelength absorption edge of Xe—Cl2—Cl mixtures (λ ≥ 309 nm), on the pressure of xenon made it possible to identify a continuum-type absorption band with a minimum at 310.5 nm. This band was attributed to the photoassociation process XeCl(X) + Xe + hν → Xe2Cl* or Xe + Cl + Xe + hν → Xe2Cl*." @default.
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- W2048654990 date "1994-03-31" @default.
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- W2048654990 title "Spectroscopic investigation of excimer molecules by photoabsorption and photoassociation methods. I. XeCl" @default.
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- W2048654990 doi "https://doi.org/10.1070/qe1994v024n03abeh000054" @default.
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