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• W2048713611 abstract "The replacement partition function was calculated for small fcc crystals by numerical normal mode analysis using exactly the same model, which considers nearest-neighbor interactions only and neglects the surface relaxation and thermal expansion, to compute all the necessary quantities. A method of calculating the surface free energy of a small crystal from data on the macroscopic surface was introduced. The numerical value of the replacement partition function thus computed was, for example, 108 at T=2θ and for n=87. This is considerably larger than the value estimated for a crystal so far, which is 102-−04 at T=2θ and for n ≅ 100. This result suggests the need of further work both in numerical calculation and in theoretical studies." @default.
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• W2048713611 date "1971-11-15" @default.
• W2048713611 modified "2023-09-27" @default.
• W2048713611 title "Replacement Partition Function for Small Crystals in Homogeneous Nucleation Theory" @default.
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• W2048713611 doi "https://doi.org/10.1063/1.1675626" @default.
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