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• W2048951908 startingPage "5235" @default.
• W2048951908 abstract "We have investigated the photofragmentation spectroscopy of Mg2(CO2)+1,2 in a reflectron time-of-flight mass spectrometer. For the linear bimolecular complex Mg2(CO2)+, we have observed three distinct molecular absorption bands, in the red, the green, and the near uv spectral regions. In each band both Mg+ and Mg+2 fragments are observed, although with different action spectra. In the uv band, we also observe reactive fragmentation to form the chemical product Mg2O+. As an initial step in investigating the dissociation mechanism and the dynamical effects which determine the final state branching, we have carried out preliminary calculations of the low lying Mg2(CO2)+ potential energy curves in collinear geometry. Photofragmentation of the complex Mg2(CO2)+2 occurs over a broad spectral range in the visible. We have found that the addition of the second solvent molecule dramatically enhances the solvent cage effect, as evidenced by a large increase in the Mg+2/Mg+ branching ratio throughout this spectral region." @default.
• W2048951908 created "2016-06-24" @default.
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• W2048951908 date "1995-04-01" @default.
• W2048951908 modified "2023-09-26" @default.
• W2048951908 title "Photofragmentation dynamics of Mg₂(CO₂)⁺_1,2" @default.
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• W2048951908 doi "https://doi.org/10.1063/1.469249" @default.
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