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- W2048982786 abstract "In this work, a block copolymer as an initiator- and monomer-free UV-cross-linked component for the controlled in situ gelation of electrolytes in dye-sensitized solar cells (DSSCs) is proposed. This block copolymer consists of one block of p-hydroxystyrene units and the other block with poly(ethylene oxide-co-propylene oxide) side chains. This block copolymer is successfully prepared by means of nitroxide-mediated polymerization, imidization reactions and successive hydrolysis reactions. When a homogeneous mixture of this copolymer and a typical liquid electrolyte (LE) is irradiated with UV, the cross-linking is efficient and controlled. The electrolyte in the DSSCs transforms in situ to a gel polymer electrolyte when exposed to UV, affording DSSCs with a relatively high initial solar-to-electricity energy conversion efficiency (η) and improved long-term stability that is significantly greater than that of the DSSCs with LE. These results demonstrate that the electrolyte system containing the UV-cross-linked block copolymer improves the long-term performance of DSSCs and contributes to the development of efficient and stable DSSCs." @default.
- W2048982786 created "2016-06-24" @default.
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- W2048982786 date "2012-01-01" @default.
- W2048982786 modified "2023-09-26" @default.
- W2048982786 title "UV-cross-linked block copolymers for initiator-free, controlled in situ gelation of electrolytes in dye-sensitized solar cells" @default.
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- W2048982786 doi "https://doi.org/10.1039/c2jm32526h" @default.
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