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- W2049590911 abstract "Experimental results are presented for one- and two-photon ionization of the water molecule, obtained using a near transform-limited xuv laser. The single-photon ionization results show rotationally resolved autoionizing resonances corresponding to members of Rydberg series (nd←1b1; n=6–11) converging on the H2O+(100) vibrational state. The two-color (1+1) multiphoton ionization results show rotationally resolved structure corresponding to Rydberg series (nd←1b1; n≥6) converging on the H2O+(000) vibrational state. Typical linewidths below and above the H2O+(000) ionization threshold are 1 and 2 cm−1, respectively. The experimental results are simulated by multichannel quantum defect theory (MQDT). The main features in the spectrum are reproduced in a treatment of the rotational channel interactions with partial l mixing. It is argued that remaining discrepancies between experiment and theory arise from perturbative interactions between the (nd←1b1) levels and members of the (nd←3a1) Rydberg series. Also, it is argued that in the (1+1) multiphoton ionization spectra lines may be missing due to selective predissociation." @default.
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- W2049590911 date "1993-02-01" @default.
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- W2049590911 title "Resonance-enhanced one- and two-photon ionization of water molecule: Preliminary analysis by multichannel quantum defect theory" @default.
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- W2049590911 doi "https://doi.org/10.1063/1.464224" @default.
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