Matches in SemOpenAlex for { <https://semopenalex.org/work/W2049604862> ?p ?o ?g. }
- W2049604862 abstract "We applied the semiclassical initial value representation method to calculate energies, lifetimes, and wave functions of scattering resonances in a two-dimensional potential for O+O2 collision. Such scattering states represent the metastable O3* species and play a central role in the process of ozone formation. Autocorrelation functions for scattering states were computed and then analyzed using the Prony method, which permits one to extract accurate energies and widths of the resonances. We found that the results of the semiclassical wave packet propagation agree well with fully quantum results. The focus was on the O16O16O18 isotopomer and the anomalous isotope effect associated with formation of this molecule, either through the O16O16+O18 or the O16+O16O18 channels. An interesting correlation between the local vibration mode character of the metastable states and their lifetimes was observed and explained. New insight is obtained into the mechanism by which the long-lived resonances in the delta zero-point energy part of spectrum produce the anomalously large isotope effect." @default.
- W2049604862 created "2016-06-24" @default.
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- W2049604862 date "2007-10-18" @default.
- W2049604862 modified "2023-09-23" @default.
- W2049604862 title "Semiclassical wave packet study of anomalous isotope effect in ozone formation" @default.
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- W2049604862 doi "https://doi.org/10.1063/1.2778432" @default.
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