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- W2050011520 abstract "Catalytic oxidation of glucose and cellulose has been demonstrated in a monolith reactor, a novel contacting device for the oxidation of carbohydrate feedstocks that allows the processing of nonsoluble components without reactor plugging. Catalytic enhancement is observed for glucose oxidation, and the catalyst promotes selectivity to two-carbon carboxylic acids. It is proposed that catalytic oxidation of glucose occurs through parallel pathways: thermal oxidation to a wide range of organic acids and selective catalytic oxidation to low molecular weight acids. On the other hand, cellulose oxidation was not always enhanced by the presence of the catalyst. Here, the effect of the catalyst was to enhance the conversion of the organic acids produced during thermal oxidation. However, these organic acids also catalyzed the primary conversion of cellulose, thus the conversion of cellulose decreased as the reaction temperature was increased. A kinetic model is provided that is consistent with the inverse temperature effect observed for the cellulose oxidation experiments." @default.
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- W2050011520 date "2000-07-14" @default.
- W2050011520 modified "2023-10-14" @default.
- W2050011520 title "Evaluation of a Monolith-Supported Pt/Al<sub>2</sub>O<sub>3</sub> Catalyst for Wet Oxidation of Carbohydrate-Containing Waste Streams" @default.
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- W2050011520 doi "https://doi.org/10.1021/es000887z" @default.
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