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- W2050125323 abstract "The orbital magnetic susceptibility (${ensuremath{chi}}_{or}^{c}$) of graphite intercalation compounds is calculated for $stackrel{ensuremath{rightarrow}}{mathrm{H}}ensuremath{parallel}stackrel{ensuremath{rightarrow}}{mathrm{c}}$ using a tight-binding model for the $ensuremath{pi}$-electron energy bands and the compact expression for ${ensuremath{chi}}_{or}^{c}$ derived by Fukuyama, which includes both intraband and interband terms. The results are presented as an approximate analytic expression for ${ensuremath{chi}}_{or}^{c}$ as a function of Fermi level $ensuremath{mu}$ ($0<ensuremath{mu}ensuremath{lesssim}3$ eV) and temperature. For $frac{ensuremath{mu}}{{k}_{B}T}ensuremath{ll}1$ the susceptibility is large and diamagnetic (due to interband transitions), while for ${k}_{B}Tensuremath{ll}ensuremath{mu}ensuremath{lesssim}3$ eV, ${ensuremath{chi}}_{or}^{c}$ is paramagnetic (mainly due to intraband transitions) in contrast to the usual Landau-Peierls diamagnetism of conduction electrons in parabolic bands. Furthermore, ${ensuremath{chi}}_{or}^{c}$ is shown to be a sensitive function of $ensuremath{mu}$ and hence of the conduction-electron charge distribution in each graphite layer. We show that this theory accounts for the main features of the experimental data (stage and temperature dependence of ${ensuremath{chi}}_{or}^{c}$) and suggest that measurements of the stage dependence of ${ensuremath{chi}}_{or}^{c}$ can be used to estimate the $c$-axis screening length in graphite intercalation compounds." @default.
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- W2050125323 date "1979-12-15" @default.
- W2050125323 modified "2023-09-30" @default.
- W2050125323 title "Theory of magnetic susceptibility of graphite intercalation compounds" @default.
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- W2050125323 doi "https://doi.org/10.1103/physrevb.20.4889" @default.
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