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• W2050176045 abstract "A theoretical description of heterogeneous charge transfer rate constants has been developed for accumulated semiconductor electrodes in contact with outer sphere redox couples. Analysis of the rate constants using a Fermi Golden Rule formalism in a non-adiabatic electron transfer framework has facilitated a theoretical comparison between the rate constants of metal and accumulated semiconductor electrodes in contact with a common electrolyte-redox couple solution. Chronoamperometric measurements of nSi electrodes in contact with CH3OH-cobaltocenium (COCp2)+-CoCp2 have been performed to investigate these predictions experimentally. A standard rate constant, k°, of (2–4) × 10−2 cm S−1 was obtained for nSi/CH3OH-CoCp2+0 contacts, while the CoCp2+0 redox couple was found to be electrochemically reversible (k° > 0.1 cm s−1) at Hg electrodes under the same conditions." @default.
• W2050176045 created "2016-06-24" @default.
• W2050176045 creator A5015008318 @default.
• W2050176045 creator A5090763304 @default.
• W2050176045 date "1996-02-01" @default.
• W2050176045 modified "2023-10-14" @default.
• W2050176045 title "Charge transfer rate constants for the reduction of cobaltocenium at accumulated nSi electrodes" @default.
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• W2050176045 doi "https://doi.org/10.1016/0020-1693(95)04881-2" @default.
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