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• W2050478841 endingPage "5042" @default.
• W2050478841 startingPage "5040" @default.
• W2050478841 abstract "This is the first report of the metal-to-ligand charge-transfer (MLCT) emission spectra of the bis-ethylenediamine- and tetraammine-bipyridineruthenium(II) complexes. The emission maxima occur at 800 and 840 nm, respectively, at 77 K in DMSO/H(2)O glasses. The MLCT excited states of these complexes have short lifetimes (less than 50 ns), and as a consequence, the emission intensities are very small. The energies of the emission maxima are very close to those expected on the basis of the difference in reduction potentials of the metal and ligand (DeltaE(1/2)) and the values of the reorganizational free energies (chi(r)) of the vertical transitions estimated from the electron-transfer self-exchange reactions of the complexes (hnu(max)(em) congruent with FDeltaE(1/2) - chi(r), where F is Faraday's constant). The low energy of the emissions is in large part a consequence of the substantial contributions of the reorganizational free energies." @default.
• W2050478841 created "2016-06-24" @default.
• W2050478841 creator A5003512483 @default.
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• W2050478841 date "2003-07-29" @default.
• W2050478841 modified "2023-10-13" @default.
• W2050478841 title "The Metal-to-Ligand Charge-Transfer Luminescences of Ruthenium(II)−Polypyridine−Tetraam(m)ine Complexes. Support for the Interconvertibility of Optical and Thermal (Kinetic) Franck−Condon Parameters" @default.
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• W2050478841 doi "https://doi.org/10.1021/ic034545g" @default.
• W2050478841 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/12924872" @default.
• W2050478841 hasPublicationYear "2003" @default.
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