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• W2050802634 abstract "Improving the catalytic activity of Pt-based bimetallic nanoparticles is a key challenge in the application of proton-exchange membrane fuel cells. Electrochemical dealloying represents a powerful approach for tuning the surface structure and morphology of these catalyst nanoparticles. We present a comprehensive study of using electrochemical dealloying methods to control the morphology of ordered Cu3Pt/C intermetallic nanoparticles, which could dramatically affect their electrocatalytic activity for the oxygen reduction reaction (ORR). Depending on the electrochemical dealloying conditions, the nanoparticles with Pt-rich core-shell or porous structures were formed. We further demonstrate that the core-shell and porous morphologies can be combined to achieve the highest ORR activity. This strategy provides new guidelines for optimizing nanoparticles synthesis and improving electrocatalytic activity." @default.
• W2050802634 created "2016-06-24" @default.
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• W2050802634 date "2015-01-22" @default.
• W2050802634 modified "2023-10-14" @default.
• W2050802634 title "Morphology and Activity Tuning of Cu₃Pt/C Ordered Intermetallic Nanoparticles by Selective Electrochemical Dealloying" @default.
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• W2050802634 doi "https://doi.org/10.1021/nl504597j" @default.
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