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- W2050872586 abstract "pH-metric and photometric investigations indicate that in the presence of excess ligand in the rare earth ion(III)-ethylenediaminetetraacetate system a binuclear complex Ln2(EDTA)36− is formed in addition to the well-known 1:1 complex LnEDTA− and the 1:2 complexes Ln(EDTA)25− and Ln(EDTA) (HEDTA)4−. With the increase of the atomic number of the rare earths the stability constants of the complexes increase up to europium, and then decrease. In the cases of ytterbium and lutetium the 1:1 complexes are the only complexes detectable. The observed trend of the stability constants can be interpreted on the basis of the decrease in size of the rare earth ions with the increase of the atomic number, and the spatial requirements of the ligand. The binuclear complex Ln2(EDTA)36− is formed from two 1:1 complex molecules; these are bridged by a third EDTA4−, the iminodiacetate groups of which each coordinate to one Ln(III)ion." @default.
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- W2050872586 date "1975-04-01" @default.
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- W2050872586 title "Equilibrium relations of rare earth ethylene-diaminetetraacetate complexes in the presence of a ligand excess" @default.
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- W2050872586 doi "https://doi.org/10.1016/0022-1902(75)80688-9" @default.
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