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• W2050876539 startingPage "11454" @default.
• W2050876539 abstract "High-pressure methods have been demonstrated to be efficient in providing new routes for the synthesis of materials of technological interest. In several molecular compounds, the drastic pressure conditions required for spontaneous transformations have been lowered to the kilobar range by photoactivation of the reactions. At these pressures, the syntheses are accessible to large-volume applications and are of interest to bioscience, space, and environmental chemistry. Here, we show that the short-lived hydroxyl radicals, produced in the photodissociation of water molecules by near-UV radiation at room temperature and pressures of a few tenths of a gigapascal (GPa), can be successfully used to trigger chemical reactions in mixtures of water with carbon monoxide or nitrogen. The detection of molecular hydrogen among the reaction products is of particular relevance. Besides the implications in fundamental chemistry, the mild pressure and irradiation conditions, the efficiency of the process, and the nature of the reactant and product molecules suggest applications in synthesis." @default.
• W2050876539 created "2016-06-24" @default.
• W2050876539 creator A5030692359 @default.
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• W2050876539 date "2009-07-14" @default.
• W2050876539 modified "2023-10-02" @default.
• W2050876539 title "High-pressure photodissociation of water as a tool for hydrogen synthesis and fundamental chemistry" @default.
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• W2050876539 doi "https://doi.org/10.1073/pnas.0901836106" @default.
• W2050876539 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/2710632" @default.
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