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- W2050910245 abstract "A model for the distribution function P(ensuremath{sigma},ensuremath{eta}) for the axial and eccentric orientational order parameters ensuremath{sigma} and ensuremath{eta} is proposed for a system of quadrupoles which represents the situation in solid ${mathrm{H}}_{2}$ and ${mathrm{D}}_{2}$. It is based on a plausible approximation to the exact one-particle orientational density matrix for J=1 molecules in the randomly distributed (J${=1)}_{X}$(J${=0)}_{(1mathrm{ensuremath{-}}X)}$ solid, where X is the molar concentration of the J=1 component. The properties of P(ensuremath{sigma},ensuremath{eta}) are described, and can be expressed as a function of a single parameter D. Three-dimensional representations of P(ensuremath{sigma},ensuremath{eta}) for several values of D are shown, where Densuremath{ll}1 and Densuremath{gg}1 represent the extreme situations for zero and complete ordering. By means of the P(ensuremath{sigma},ensuremath{eta}) model, the NMR line shape for an ortho-para-mixture polycrystalline sample is calculated and compared with experiments in ${mathrm{H}}_{2}$. The correlation of the parameter D with a given ordering state in the temperature-concentration plane for ${mathrm{H}}_{2}$, the effect of zero-point motion, and the effect of crystalline anisotropy on the line shape are discussed." @default.
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- W2050910245 date "1988-03-01" @default.
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- W2050910245 title "Distribution function for the orientational order parameters in solidH2andD2" @default.
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- W2050910245 doi "https://doi.org/10.1103/physrevb.37.3216" @default.
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