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- W2051109747 abstract "Abstract The catalyst performance of MoS 2 and WS 2 was verified for the CO 2 -reforming of CH 4 through the comparison with that of Ni SiO 2 . No catalyst deactivation was observed on the disulfides, although the rate was much smaller than that on Ni. It was found that the disulfides exhibited a poor ability for the direct decomposition of CH 4 . The poor ability did not lead to carbon deposition during reforming reaction, which assured a stable activity. It was also observed that the rate equation was completely different between disulfide catalysts and Ni catalyst. The reaction order was positive with respect to the CH 4 partial pressure and negative with respect to the CO 2 partial pressure on the former catalysts, while negative with respect to CH 4 partial pressure and positive with respect to the CO 2 partial pressure on the latter. The observed reaction kinetics suggested that the surface of the disulfide catalyst was abundant in adsorbed CO 2 , while the surface of Ni catalyst was abundant in adsorbed CH 4 . The abundance in adsorbed CO 2 was considered an unfavorable condition for the direct decomposition of CH 4 and as a result, carbon deposition was suppressed during CO 2 -reforming on disulfide catalyst. Sulfur tolerance was found to be an additional performance of the disulfide catalyst." @default.
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- W2051109747 date "1997-07-01" @default.
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- W2051109747 title "Catalyst performance of MoS2 and WS2 for the CO2-reforming of CH4 Suppression of carbon deposition" @default.
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- W2051109747 doi "https://doi.org/10.1016/s0926-860x(96)00391-2" @default.
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