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• W2051200838 abstract "Recently, Maitlis et al. [J. Catal. 167 (1997) 172] proposed an alternative reaction pathway for chain growth in the Fischer–Tropsch synthesis. In this mechanism, chain growth is assumed to occur by methylene insertion into a metal–vinyl bond, forming an allyl species that will subsequently isomerise to a vinyl species. Organo-metallic allyl complexes, Fe{[η5-C5H5](CO)2CH2CHCH2} and Fe{[η5-C5(CH3)5](CO)2CH2CHCH2} were synthesised. Under thermal treatment, the decomposition of these complexes was observed, instead of the isomerisation. In a hydrogen atmosphere, the reduction of the iron–carbon bonds and the hydrogenation yielding iron–alkyl species was observed. This clearly shows that the proposed vinyl–allyl isomerisation is unlikely to occur in mono-nuclear iron complexes. Hence, it might be expected that the reaction mechanism proposed by Maitlis et al. [J. Catal. 167 (1997) 172] is unlikely to be the main route for chain growth in the Fischer–Tropsch synthesis." @default.
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• W2051200838 date "2002-01-01" @default.
• W2051200838 modified "2023-10-14" @default.
• W2051200838 title "Some evidence refuting the alkenyl mechanism for chain growth in iron-based Fischer–Tropsch synthesis" @default.
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• W2051200838 doi "https://doi.org/10.1016/s0920-5861(01)00461-8" @default.
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