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- W2051205221 abstract "We propose a generalized one-dimensional energy diffusion approach for describing the dynamics of multidimensional dynamical processes in the condensed phase. On the basis of a formalism originally due to Zwanzig, we obtain a one-dimensional kinetic equation for a properly selected relevant dynamical quantity and derive new analytical results for the dynamics of a multidimensional electron-transfer process, nonequilibrium solvation, and diffusive escape from a potential well. The calculated results for electron-transfer reactions in solvent-separated and contact ion pair systems are found to be in good agreement with the experimental results. We are able to explain the rate of the electron-transfer reaction using much smaller and reasonable values of the solvent reorganization energy in contrast to earlier works that had to use a much larger value. The proposed theory is not only conceptually simpler than the conventional approaches but is also free from many of their limitations. More importantly, it provides a single theoretical framework for describing a wide class of dynamical phenomena." @default.
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- W2051205221 date "2008-01-01" @default.
- W2051205221 modified "2023-09-23" @default.
- W2051205221 title "A One-Dimensional Energy Diffusion Approach to Multidimensional Dynamical Processes in the Condensed Phase" @default.
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- W2051205221 doi "https://doi.org/10.1021/jp076954u" @default.
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