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• W2051216538 abstract "We present photoelectron spectroscopy studies on Znn− in the size range of n=3–117. We show that zinc clusters exhibit a distinct transition in their electronic structure as a function of size. At small sizes (up to n=18) the clusters follow the Bloch-Wilson picture of the development of a metal from closed-shell atoms, exhibiting a gradual decrease of the gap between the fully occupied s band and the empty p band. For large sizes (n≳32) the band overlap allows the valence electrons to fully delocalize. This leads to an almost perfect free-electron density of states, as is demonstrated by discussing the spectra in the light of standard free-electron models and by comparison to the results obtained on sodium clusters." @default.
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• W2051216538 date "2005-12-08" @default.
• W2051216538 modified "2023-09-27" @default.
• W2051216538 title "Transition from a Bloch-Wilson to a free-electron density of states in Znn− clusters" @default.
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• W2051216538 doi "https://doi.org/10.1063/1.2138689" @default.
• W2051216538 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16375459" @default.
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