FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2051217648> ?p ?o ?g. }

• W2051217648 endingPage "19633" @default.
• W2051217648 startingPage "19623" @default.
• W2051217648 abstract "The relationship between spatially heterogeneous dynamics (SHD) and jamming is studied in a glass-forming binary Lennard-Jones system via molecular dynamics simulations. It has been suggested [Phys. Rev. Lett. 2001, 86, 111]1 that the probability distribution of interparticle forces P(F) develops a peak at the glass transition temperature Tg and that the large force inhomogeneities, responsible for structural arrest in granular materials, are related to dynamical heterogeneities in supercooled liquids that form glasses. It has been further suggested that “force chains” present in granular materials may exist in supercooled liquids and may provide an order parameter for the glass transition. Our goal is to investigate the extent to which the forces experienced by particles in a glass-forming liquid are related to SHD and compare these forces to those observed in granular materials and other glass-forming systems. Our results are summarized as follows. We calculate P(F) for positive (repulsive) instantaneous forces and find no peak in P(F) at any temperature in our system, even below Tg. We also find that particles that have been localized for a long time are less likely to experience high relative force and that mobile particles experience higher relative forces at shorter time scales, indicating a correlation between pairwise forces and particle mobility. We construct force chains based on the magnitude of pairwise positive instantaneous forces. We find that force chains constructed in this manner are composed of both localized and mobile particles; therefore there is no one-to-one correspondence between force chains as defined here and locally mobile or immobile regions of the liquid. We also find that force chains do not play the same role as force chains in granular materials but may indicate a difference in the evolution of the local environment of particles with different mobility. We also discuss a possible relationship between force chains found here and the development of stringlike motion found in this and other glass-forming liquids [Phys. Rev. Lett. 1998, 80, 2338; J. Chem. Phys. 2004, 120, 4415].2,3" @default.
• W2051217648 created "2016-06-24" @default.
• W2051217648 creator A5045900230 @default.
• W2051217648 creator A5078375520 @default.
• W2051217648 date "2004-12-01" @default.
• W2051217648 modified "2023-09-26" @default.
• W2051217648 title "Dynamical Heterogeneity and Jamming in Glass-Forming Liquids" @default.
• W2051217648 cites W1555502983 @default.
• W2051217648 cites W1646671735 @default.
• W2051217648 cites W1966504366 @default.
• W2051217648 cites W1971782949 @default.
• W2051217648 cites W1974178725 @default.
• W2051217648 cites W1974195642 @default.
• W2051217648 cites W1974563879 @default.
• W2051217648 cites W1980144709 @default.
• W2051217648 cites W1983512333 @default.
• W2051217648 cites W1989805067 @default.
• W2051217648 cites W1991178580 @default.
• W2051217648 cites W1991968342 @default.
• W2051217648 cites W1997992337 @default.
• W2051217648 cites W1999183541 @default.
• W2051217648 cites W2004967763 @default.
• W2051217648 cites W2010478552 @default.
• W2051217648 cites W2012422733 @default.
• W2051217648 cites W2012629131 @default.
• W2051217648 cites W2015125017 @default.
• W2051217648 cites W2015837502 @default.
• W2051217648 cites W2016366045 @default.
• W2051217648 cites W2020922425 @default.
• W2051217648 cites W2021195194 @default.
• W2051217648 cites W2021641921 @default.
• W2051217648 cites W2022131461 @default.
• W2051217648 cites W2022220643 @default.
• W2051217648 cites W2022861351 @default.
• W2051217648 cites W2022923036 @default.
• W2051217648 cites W2023305433 @default.
• W2051217648 cites W2024649065 @default.
• W2051217648 cites W2026120411 @default.
• W2051217648 cites W2027154261 @default.
• W2051217648 cites W2027718072 @default.
• W2051217648 cites W2027840351 @default.
• W2051217648 cites W2027923654 @default.
• W2051217648 cites W2031715663 @default.
• W2051217648 cites W2034875509 @default.
• W2051217648 cites W2040179043 @default.
• W2051217648 cites W2040679855 @default.
• W2051217648 cites W2041679326 @default.
• W2051217648 cites W2042399894 @default.
• W2051217648 cites W2046645394 @default.
• W2051217648 cites W2047616041 @default.
• W2051217648 cites W2048458072 @default.
• W2051217648 cites W2055166044 @default.
• W2051217648 cites W2060475636 @default.
• W2051217648 cites W2062232020 @default.
• W2051217648 cites W2063039567 @default.
• W2051217648 cites W2064430530 @default.
• W2051217648 cites W2065674696 @default.
• W2051217648 cites W2068493779 @default.
• W2051217648 cites W2071688608 @default.
• W2051217648 cites W2074252130 @default.
• W2051217648 cites W2077058849 @default.
• W2051217648 cites W2080611207 @default.
• W2051217648 cites W2080911709 @default.
• W2051217648 cites W2084420590 @default.
• W2051217648 cites W2090216453 @default.
• W2051217648 cites W2090633257 @default.
• W2051217648 cites W2093273986 @default.
• W2051217648 cites W2093694187 @default.
• W2051217648 cites W2094596736 @default.
• W2051217648 cites W2096848392 @default.
• W2051217648 cites W2105479026 @default.
• W2051217648 cites W2132087474 @default.
• W2051217648 cites W2135835362 @default.
• W2051217648 cites W2138971677 @default.
• W2051217648 cites W2143566629 @default.
• W2051217648 cites W2145479290 @default.
• W2051217648 cites W2158195839 @default.
• W2051217648 cites W2162901662 @default.
• W2051217648 cites W2170797104 @default.
• W2051217648 cites W2542397303 @default.
• W2051217648 doi "https://doi.org/10.1021/jp040401r" @default.
• W2051217648 hasPublicationYear "2004" @default.
• W2051217648 type Work @default.
• W2051217648 sameAs 2051217648 @default.
• W2051217648 citedByCount "22" @default.
• W2051217648 countsByYear W20512176482012 @default.
• W2051217648 countsByYear W20512176482013 @default.
• W2051217648 countsByYear W20512176482014 @default.
• W2051217648 countsByYear W20512176482015 @default.
• W2051217648 countsByYear W20512176482018 @default.
• W2051217648 countsByYear W20512176482021 @default.
• W2051217648 countsByYear W20512176482022 @default.
• W2051217648 crossrefType "journal-article" @default.
• W2051217648 hasAuthorship W2051217648A5045900230 @default.
• W2051217648 hasAuthorship W2051217648A5078375520 @default.
• W2051217648 hasBestOaLocation W20512176482 @default.
• W2051217648 hasConcept C111368507 @default.
• W2051217648 hasConcept C112964491 @default.

• next