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• W2051228679 abstract "The first total synthesis of (+)-frondosin A was accomplished in 19 longest linear and 21 total steps from commercially available materials. The key features of the synthesis include a Ru-catalyzed [5+2] cycloaddition, a Claisen rearrangement, and a ring expansion to construct the core of the frondosin A in a diastereoselective and regioselective fashion. This is the first application of a Ru-catalyzed [5+2] cycloaddition in the total synthesis of a natural product. Through this synthesis, the absolute configuration of (+)-frondosin A was established." @default.
• W2051228679 created "2016-06-24" @default.
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• W2051228679 date "2007-08-31" @default.
• W2051228679 modified "2023-10-11" @default.
• W2051228679 title "Total Synthesis of (+)-Frondosin A. Application of the Ru-Catalyzed [5+2] Cycloaddition" @default.
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• W2051228679 doi "https://doi.org/10.1021/ja073272b" @default.
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