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• W2051230328 abstract "We have synthesized new wholly aromatic polymers containing hemicyanine dyes in the side chain. The polymers are soluble in both protic solvents (methanol, ethanol, phenol) and aprotic solvents (DMSO, NMP, DMAc). However, they could not be processed into good optical quality films by simple casting or spin-coating. These amphiphilic polymers exhibited a polyelectrolyte effect in deionized water. The excessive positive charges along the hydrophobic rigid backbones, which bear two charged groups per repeat unit at the end of the methylene spacers, dramatically affect their dimension in solution, with intramolecular charge repulsions tending to assume an extended conformation. The bulk susceptibility of these materials was determined by the second harmonic generation technique. Significant SHG activity was observed from the spin-coated films without the aid of electric field induced poling. However, the corona-poled polymer films showed smaller d33 values in the range 70−105 pm/V than expected due to the inefficient electric poling, which we discuss in terms of the domains of the chromophores that are not well developed by electric poling." @default.
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• W2051230328 date "2000-11-16" @default.
• W2051230328 modified "2023-10-10" @default.
• W2051230328 title "New Amphiphilic Rodlike Polymers with Pendent Hemicyanine Groups. 1. Synthesis and Properties" @default.
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• W2051230328 doi "https://doi.org/10.1021/ma0010938" @default.
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