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• W2051240721 abstract "The role of band bending on the efficiency of charge transfer across the TiO2(110) single crystal surface has been measured in ultrahigh vacuum, in the absence of a wide range of surface site inhomogeneities, surface impurities and solvent effects, and particle size effects. The adsorption of the Cl2 (electron acceptor) molecule and the O2 (electron acceptor) molecule have been found to enhance hole transport from TiO2 to 18O2 molecules adsorbed on oxygen vacancy sites, increasing the rate of electron stimulated desorption (ESD) of 18O2. This confirms that O2-ESD is hole mediated. Conversely, adsorption of CH3OH, a donor molecule, reduces the transfer rate for holes to the adsorbed O2, reducing its rate of ESD to near zero. The maximum effect of donor and acceptor molecules occurs near 1 monolayer coverage." @default.
• W2051240721 created "2016-06-24" @default.
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• W2051240721 creator A5061083189 @default.
• W2051240721 date "2010-07-01" @default.
• W2051240721 modified "2023-09-27" @default.
• W2051240721 title "Effect of Adsorbed Donor and Acceptor Molecules on Electron Stimulated Desorption: O₂/TiO₂(110)" @default.
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• W2051240721 doi "https://doi.org/10.1021/jz1007559" @default.
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