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• W2051244146 abstract "Shibasaki's heterobimetallic complexes M3(THF)n(BINOLate)3Ln [M = Li, Na, K; Ln = lanthanide(III)] are among the most successful asymmetric Lewis acid catalysts. Why does M3(THF)n(BINOLate)3Ln readily bind substrates when M = Li but not when M = Na or K? Structural studies herein indicate Na− and K−C cation−π interactions and alkali metal radius may be more important than even lanthanide radius. Also reported is a novel polymeric [K3(THF)2(BINOLate)3Yb]n structure that provides the first evidence of interactions between M3(THF)n(BINOLate)3Ln complexes." @default.
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• W2051244146 date "2007-07-21" @default.
• W2051244146 modified "2023-10-03" @default.
• W2051244146 title "Impact of Na− and K−C π-Interactions on the Structure and Binding of M₃(sol)<i>_n</i>(BINOLate)₃Ln Catalysts" @default.
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• W2051244146 doi "https://doi.org/10.1021/ol0713234" @default.
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