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- W2051325661 abstract "Polarized absorption spectra of single crystals of LiClO4· 3H2O/LiMnO4· 3H2O and Ba(ClO4)2· 3H2O/Ba(MnO4)2· 3H2O have been measured at 4.2°K in the region λ>5800 Å. The transition whose ⊥ components possess zero-phonon origins at 13774 cm−1 in the lithium salt and at 14247 cm−1 in the barium salt is unequivocally identified as an electric-dipole forbidden T11←A11 transition of the parent tetrahedral point group. In the C3v site symmetry of the lithium salt the ⊥ component of this transition is shown to be electric-dipole allowed; in the C3 site symmetry of the barium salt the crystallographic site-splitting of the ⊥ and ‖ components is 152 cm−1, and both component transitions are shown to be electric-dipole allowed. It is deduced that both the far-red transition and the 5200-Å absorption band of permangante ion arise dominantly from e↔ t1 or e↔ t2 single-configurational excitations. A discussion of the extensive phonon coupling and the anomalous Franck—Condon pattern of this transition is also provided." @default.
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- W2051325661 date "1971-11-01" @default.
- W2051325661 modified "2023-09-23" @default.
- W2051325661 title "Electronic Absorption Spectrum of MnO4− in the Far-Red Region" @default.
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- W2051325661 doi "https://doi.org/10.1063/1.1676776" @default.
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