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• W2051551137 abstract "Unimolecular decay rates and monomer-dimer branching ratios of gold clusters ${{mathrm{Au}}_{N}}^{+}$ $(N=7--27)$ have been measured as a function of excitation energy in photodissociation experiments on size-selected clusters stored in a Penning trap. Part of the data set has previously been used to extract model-free values of dissociation energies [Vogel et al., Phys. Rev. Lett. 87, 013401 (2001)]. Other parts of the data set do not allow this analysis. We use these data to extract tentative dissociation energies, based on the systematics of deviations between an Arrhenius analysis and the model-free values. The observed systematics also allows an estimate of the true frequency factor which often is much higher than the Arrhenius value but in good agreement with the expected detailed balance value. The data are also reanalyzed including radiative cooling which may explain part of the discrepancy between model-free and Arrhenius dissociation-energy values." @default.
• W2051551137 created "2016-06-24" @default.
• W2051551137 creator A5012159432 @default.
• W2051551137 creator A5041415843 @default.
• W2051551137 creator A5071640860 @default.
• W2051551137 creator A5073515528 @default.
• W2051551137 date "2006-06-13" @default.
• W2051551137 modified "2023-10-02" @default.
• W2051551137 title "Dissociation energies of gold clusters<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:msub><mml:mi mathvariant=normal>Au</mml:mi><mml:mi>N</mml:mi></mml:msub><mml:mo>+</mml:mo></mml:msup></mml:mrow></mml:math>,<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi>N</mml:mi><mml:mo>=</mml:mo><mml:mn>7</mml:mn><mml:mo>–</mml:mo><mml:mn>27</mml:mn></mml:mrow></mml:math>" @default.
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• W2051551137 doi "https://doi.org/10.1103/physreva.73.063202" @default.

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