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- W2051551820 abstract "A semi-classical treatment of the non-adiabatic among a set of several interacting states is presented. The electrons are described by a wave function obtained by the integration of a set of coupled differential equations. An expression for the force acting on the nuclei is obtained by requiring the total energy to remain constant. This force is found to be equal to the sum of two contributions. The first one is the average of the forces deriving from each Born-Oppenheimer potential. The second one is an interference term which exhibits oscillations in a region of strong non-adiabatic coupling and vanishes outside. An application to a set of fourteen states of a diatomic molecule is presented. The results are sometimes at variance with those predicted by the Landau-Zener equation." @default.
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- W2051551820 date "1975-06-01" @default.
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- W2051551820 title "Non-adiabatic interactions in unimolecular decay. I" @default.
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- W2051551820 doi "https://doi.org/10.1016/0301-0104(75)80124-8" @default.
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