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- W2051687236 abstract "The relevance of stochastic effects at very low template concentration for Qs-catalized-template-instructed RNA replication is established. The fluctuations in rates and in elongation intermediate concentrations are determined making use of a center manifold stochastic reduction of the fast-relaxing kinetic degrees of freedom. The strength of these far-from-equilibrium fluctuations is scaled with the small rate-control characteristic parameters of the system. The fluctuations in the concentration of the chain-elongation intermediate complexes are enhanced as the template chain becomes shorter, thus, a deterministic description does not hold for RNA chains of the order of 50 nucleotides. Some results on the de-novo synthesis of RNA are reinterpreted in the light of these experimental findings. The far-from-equilibrium fluctuations determine the scattering of lag-times corresponding to the macroscopically-detectable amplification of the template. The results show very good agreement with the experimental evidence." @default.
- W2051687236 created "2016-06-24" @default.
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- W2051687236 date "1987-10-01" @default.
- W2051687236 modified "2023-09-26" @default.
- W2051687236 title "Intrinsic Fluctuations in Macromolecular Self-Replicating Systems" @default.
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- W2051687236 doi "https://doi.org/10.1002/bbpc.19870911005" @default.
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