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- W2051838441 abstract "We have developed new techniques for measuring infrared spectra at megabar pressures using synchrotron radiation and applied them to study the ${mathit{Q}}_{1}$(1), ${mathit{Q}}_{1}$(1)+${mathit{S}}_{1}$(0), and ${mathit{Q}}_{mathit{R}}$(J) vibrational transitions of solid hydrogen to 180 GPa. The frequency difference between the ${mathit{Q}}_{1}$(1) infrared and Raman vibrons increases from 3 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$ (zero pressure) to 510 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$ (180 GPa), including a dramatic increase in intermolecular coupling with pressure. A negative frequency shift is observed for the infrared vibron above 140 GPa. A significant increase in frequency and LO-TO splitting of the lattice phonon is also documented." @default.
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- W2051838441 date "1992-08-17" @default.
- W2051838441 modified "2023-10-13" @default.
- W2051838441 title "Synchrotron infrared spectroscopy at megabar pressures: Vibrational dynamics of hydrogen to 180 GPa" @default.
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- W2051838441 doi "https://doi.org/10.1103/physrevlett.69.1129" @default.
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