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• W2051898940 startingPage "8847" @default.
• W2051898940 abstract "Metathesis reactions between Ru(2)(DMBA)(4)Cl(2) (DMBA = N,N'-dimethylbenzamidinate) and MX (M = Na and K) yielded bis-adduct derivatives Ru(2)(DMBA)(4)X(2) (X = CN (1), N(3) (2), N(CN)(2) (3)). Metathesis reactions between Ru(2)(DMBA)(4)(NO(3))(2) and KI resulted in Ru(2)(DMBA)(4)I(2) (4). Compound 1 is diamagnetic, while compounds 2-4 are paramagnetic (S = 1). Both compounds 1 and 2 undergo two reversible one-electron processes, an oxidation and a reduction, while compound 3 features a quasireversible reduction. Single-crystal X-ray diffraction studies revealed that the Ru-Ru bond lengths are 2.4508(9), 2.3166(7), 2.304[1], and 2.328(1) A for compounds 1-4, respectively. Structural and electrochemical data clearly indicate that the axial ligands impart a significant influence on the electronic structures of diruthenium species." @default.
• W2051898940 created "2016-06-24" @default.
• W2051898940 creator A5025013285 @default.
• W2051898940 creator A5059304767 @default.
• W2051898940 date "2003-11-13" @default.
• W2051898940 modified "2023-10-16" @default.
• W2051898940 title "Synthesis and Characterization of Ru₂(DMBA)₄X₂ (X = CN, N₃, N(CN)₂, I): Controlling Structural, Redox, and Magnetic Properties with Axial Ligands" @default.
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• W2051898940 doi "https://doi.org/10.1021/ic035106k" @default.
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