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- W2051918206 abstract "Abstract The endothermic decomposition of metal pyrosulfate in molten phase to produce metal sulfate and sulfur trioxide gas is an important chemical energy storage reaction. A chemical reaction engineering analysis of certain literature data was carried out to obtain a model for the decomposition and the rate constant as a function of temperature. The analysis indicates that the rate controlling reaction event is the cation-anion interaction of K+ and S2O7−2 ions to form KS2O7−1, simultaneously polarizing the latter to weaken the SOS bridge and release SO3. Based on this view transition state theory was applied and yielded an expression for the rate constant in essential agreement with experimental data. A preliminary model for a pilot-scale reactor is presented." @default.
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- W2051918206 date "1986-01-01" @default.
- W2051918206 modified "2023-09-24" @default.
- W2051918206 title "Chemical storage of solar energy—The Flood-Förland-Lindemann hypotheses and the decomposition of pyrosulfate ions" @default.
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- W2051918206 doi "https://doi.org/10.1016/0038-092x(86)90046-0" @default.
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